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All-Optically Controlled Memristor

Lingxiang Hu, Jing Yang, Jingrui Wang, Peihong Cheng, Leon O. Chua, Fei Zhuge

arXiv:2004.08077v1cond-mat.mtrl-sciphysics.app-ph

TL;DR

The paper examines bilayered IGZO memristive switching, where the interfacial region plays a key role. It attributes switching to oxygen-vacancy electron trapping and detrapping and demonstrates synaptic potentiation with MC1 > MC2 and ΔW1 > ΔW2.

  • Problem

    Bilayered OD-IGZO/OR-IGZO memristive switching requires identifying the roles of its interfacial region and memconductance dependence.

  • Method

    The paper attributes switching in bilayered OD-IGZO/OR-IGZO devices to electron trapping and detrapping at ionized or neutral oxygen vacancies.

  • Results

    Near-infrared stimulation realizes synaptic potentiation, with MC1 > MC2 and ΔW1 > ΔW2.

  • Takeaways & Limitations

    The device supports optical emulation of synaptic potentiation through controlled memconductance updates.

Abstract

from arXiv · show

Memristors have emerged as key candidates for beyond-von-Neumann neuromorphic or in-memory computing owing to the feasibility of their ultrahigh-density three-dimensional integration and their ultralow energy consumption. A memristor is generally a two-terminal electronic element with conductance that varies nonlinearly with external electric stimuli and can be remembered when the electric power is turned off. As an alternative, light can be used to tune the memconductance and endow a memristor with a combination of the advantages of both photonics and electronics. Both increases and decreases in optically induced memconductance have been realized in different memristors; however, the reversible tuning of memconductance with light in the same device remains a considerable challenge that severely restricts the development of optoelectronic memristors. Here we describe an all-optically controlled (AOC) analog memristor with memconductance that is reversibly tunable over a continuous range by varying only the wavelength of the controlling light. Our memristor is based on the relatively mature semiconductor material InGaZnO (IGZO) and a memconductance tuning mechanism of light-induced electron trapping and detrapping. We demonstrate that spike-timing-dependent plasticity (STDP) learning can be realized in our device, indicating its potential applications in AOC spiking neural networks (SNNs) for highly efficient optoelectronic neuromorphic computing.

Methods

The study fabricated amorphous OD-IGZO/OR-IGZO bilayer devices with Au or ITO electrodes and characterized their structural, electrical, optical, and electronic properties. The bilayer interface governs memristive switching through oxygen-vacancy electron trapping and detrapping, while RESET establishes a reproducible low-memconductance state.

  • Material characterization: Hall measurements showed OD-IGZO at 1019 cm−3 and 10−2 Ωcm, whereas OR-IGZO exceeded the measurement limit of approximately 105 Ωcm.The conductivity contrast indicates substantially different oxygen-vacancy densities between the two films.
  • Electronic characterization: Optical and photoelectron measurements determined band gaps of 3.7 and 3.6 eV and work functions of 4.2 and 4.9 eV for OD-IGZO and OR-IGZO, respectively.The corresponding EF–EV values were 3.1 and 2.5 eV from XPS, consistent with UPS values of 3.2 and 2.6 eV.
  • Device mechanism: OD-IGZO/OR-IGZO interfacial regions play a key role in memristive switching, with memconductance attributed to electron trapping and detrapping at oxygen vacancies.The bilayer showed pronounced I–V differences from single-layer devices, supporting an interfacial switching origin.

Data availability

The data supporting this study’s findings are available from the corresponding authors.

  • Data availability: Study data supporting the findings are available from the corresponding authors.
  • Data availability: The corresponding authors provide access to the data supporting the study’s findings.
  • Data availability: Data availability is directed through the study’s corresponding authors.

Additional information

The additional information documents the device’s OD-IGZO/OR-IGZO structure, band alignment, switching characteristics, optical/electrical control, and STDP-emulation mechanism through extended data.

  • Device structure: Extended Data Fig. 1 characterizes the Au/OD-IGZO/OR-IGZO/Pt device structure and the boundary between the two IGZO layers using TEM and HRTEM images.The device is deposited on Pt/Ti/SiO2/Si, and FFT images are provided for the high-resolution micrograph.
  • Memristive switching: Extended Data Fig. 2 reports retention of the low- and high-memconductance states and reversible conductance regulation using positive SET and negative RESET voltage pulses.The pulses have 2 V amplitude, 25 ms duration, and 250 ms intervals; conductance is measured at 10 mV.
  • Mechanism analysis: Extended Data Figs. 3 and 4 analyze the OD-IGZO/OR-IGZO band structure and the memristive switching mechanism using optical, photoelectron, electrical, and device-size measurements.The supplied band parameters include OD-IGZO EF−EV = 3.1 eV, OR-IGZO EF−EV = 2.5 eV, and OR-IGZO Eg = 3.6 eV.
  • STDP mechanism: Extended Data Fig. 9 explains STDP emulation: positive timing differences produce potentiation, negative timing differences produce depression, and shorter intervals yield larger weight changes.For potentiation, ΔW1 > ΔW2; for depression, |ΔW1| > |ΔW2| under the specified timing conditions.
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